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Yang, Chi-Yuan ; Stoeckel, Marc-Antoine ; Ruoko, Tero-Petri ; Wu, Han-Yan ; Liu, Xianjie ; Kolhe, Nagesh B. ; Wu, Ziang ; Puttisong, Yuttapoom ; Musumeci, Chiara ; Massetti, Matteo ; et al ( , Nature Communications)
Abstract Conducting polymers, such as the
p -doped poly(3,4-ethylenedioxythiophene):poly(styrene sulfonate) (PEDOT:PSS), have enabled the development of an array of opto- and bio-electronics devices. However, to make these technologies truly pervasive, stable and easily processable,n -doped conducting polymers are also needed. Despite major efforts, non -type equivalents to the benchmark PEDOT:PSS exist to date. Here, we report on the development of poly(benzimidazobenzophenanthroline):poly(ethyleneimine) (BBL:PEI) as an ethanol-basedn -type conductive ink. BBL:PEI thin films yield ann -type electrical conductivity reaching 8 S cm−1, along with excellent thermal, ambient, and solvent stability. This printablen -type mixed ion-electron conductor has several technological implications for realizing high-performance organic electronic devices, as demonstrated for organic thermoelectric generators with record high power output andn -type organic electrochemical transistors with a unique depletion mode of operation. BBL:PEI inks hold promise for the development of next-generation bioelectronics and wearable devices, in particular targeting novel functionality, efficiency, and power performance. -
Xu, Kai ; Sun, Hengda ; Ruoko, Tero-Petri ; Wang, Gang ; Kroon, Renee ; Kolhe, Nagesh B. ; Puttisong, Yuttapoom ; Liu, Xianjie ; Fazzi, Daniele ; Shibata, Koki ; et al ( , Nature Materials)